J. Karl Johnson
Professor, Department of Chemical and Petroleum Engineering
1242 Benedum Hall
412-624-5644, 9639(fax)
karlj@engr.pitt.edu
http://puccini.che.pitt.edu/index.html
Control of materials at the atomic scale often involves
confinement of molecules to nanometer-size domains. We have
developed an extensive research program to describe the
equilibrium and transport properties of fluids confined in
nanoporous materials, such as single walled carbon nanotubes and
metal organic frameworks. Nano-confined fluids may exhibit very
different behavior from bulk fluids. For example, we have
predicted quantum sieving of isotopes, extremely high transport
rates of fluids in carbon nanotubes, and unique hydrogen bonding
of confined water. Manipulation of structures and properties at
the nanoscale will lead to the development of new processes and
products.

|
Water molecules confined inside a single
walled carbon nanotube: The water molecules adopt a
stacked-ring structure, bound by two different types of
hydrogen bonding. Hydrogen atoms that participate in
intra-ring hydrogen bonding are colored green while
inter-ring hydrogen bonding is shown by the blue atoms. |